The global shift toward low-carbon energy and circular chemical manufacturing is driving the demand for heterogeneous catalysts that can efficiently convert sustainable feedstocks into target chemicals. Zeolites, with their flexible frameworks, tunable acidity, and metal site environments, are poised to play a pivotal role in the green energy revolution. Beyond their traditional role as acid catalysts in petroleum refining, zeolites are opening new routes for converting low-carbon molecules such as CH4 and CO2, upgrading biomass-derived oxygenates, and upcycling waste plastics. Achieving these goals requires greener and more efficient synthesis routes for zeolites with desired topologies, controlled active sites, and improved accessibility. In this perspective, recent advances in the green and efficient synthesis of zeolites with tailored framework topologies will be introduced first. Next, the synthetic approaches of multifunctional zeolite catalysts will be highlighted. Furthermore, predictive synthesis combining computational modeling and machine learning is facilitating the rational design of zeolite catalysts for green energy applications. These developments illustrate how engineering zeolite synthesis can lead to efficient catalytic processes for producing fuels and chemicals from sustainable feedstocks.